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Aller au contenu ChemDigest Menu principal Cobalt Single Atoms Anchored on Oxygen‐Doped Tubular Carbon Nitride for Efficient Peroxymonosulfate Activation: Simultaneous Coordination Structure and Morphology Modulation Par admin / 26 mai 2022 26 mai 2022 / Non classé A synthetic method was developed to modulate the coordination environment and regulate support architecture, thus incorporating oxygen atoms into the first shell of Co single-atom catalysts (SACs). The high activity and 1 O 2 selectivity of Co−N 3 O 1 correlated with an enhanced adsorption energy of peroxymonosulfate (PMS) and reduced activation barriers. As a result, the catalysts were attached to a membrane to deliver a catalytic filter with 97.5 % ciprofloxacin rejection over 10 hours. Abstract Simultaneous regulation of the coordination environment of single-atom catalysts (SACs) and engineering architectures with efficient exposed active sites are efficient strategies for boosting peroxymonosulfate (PMS) activation. We

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